دورية أكاديمية

Global and regional chemical influence of sprites: reconciling modelling results and measurements

التفاصيل البيبلوغرافية
العنوان: Global and regional chemical influence of sprites: reconciling modelling results and measurements
المؤلفون: F. J. Pérez-Invernón, F. J. Gordillo-Vázquez, A. Malagón-Romero, P. Jöckel
المصدر: Atmospheric Chemistry and Physics, Vol 24, Pp 3577-3592 (2024)
بيانات النشر: Copernicus Publications, 2024.
سنة النشر: 2024
المجموعة: LCC:Physics
LCC:Chemistry
مصطلحات موضوعية: Physics, QC1-999, Chemistry, QD1-999
الوصف: Mesospheric electrical discharges, known as sprites and formed by fast-propagating streamers, have been shown to create localized enhancements of atmospheric constituents such as N, O, NOx, N2O, and HOx, as indicated by both modelling results and space-based measurements. In this study, we incorporate the occurrence rate of sprites into a chemistry–climate model using meteorological parameters as a proxy. Additionally, we introduce the injection of chemical species by sprites into the model based on electrodynamical modelling of individual sprite streamers and observations from space. Our modelling results show a good agreement between the simulated sprite distribution and observed data on a global scale. While the global influence of sprites on the atmospheric chemistry is found to be negligible, our findings reveal their measurable chemical influence at the regional scale, particularly for the concentration of HNO3 and HNO4 within the mesosphere. The simulations also suggest that sprites could be responsible for the observed NO2 anomalies at an altitude of 52 km above thunderstorms, as reported by MIPAS. Finally, a projected simulation reveals that the occurrence rate of sprites could increase at a rate of 14 % per 1 K rise in the global temperature.
نوع الوثيقة: article
وصف الملف: electronic resource
اللغة: English
تدمد: 1680-7316
1680-7324
العلاقة: https://acp.copernicus.org/articles/24/3577/2024/acp-24-3577-2024.pdfTest; https://doaj.org/toc/1680-7316Test; https://doaj.org/toc/1680-7324Test
DOI: 10.5194/acp-24-3577-2024
الوصول الحر: https://doaj.org/article/698c6d95a8c246dc8292952e2d0df463Test
رقم الانضمام: edsdoj.698c6d95a8c246dc8292952e2d0df463
قاعدة البيانات: Directory of Open Access Journals
الوصف
تدمد:16807316
16807324
DOI:10.5194/acp-24-3577-2024