دورية أكاديمية
Facile Synthesis of Unsupported Pd Aerogel for High Performance Formic Acid Microfluidic Fuel Cell
| العنوان: | Facile Synthesis of Unsupported Pd Aerogel for High Performance Formic Acid Microfluidic Fuel Cell |
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| المؤلفون: | Martínez-Lázaro, Alejandra, Ramírez Montoya, Luis Adrián, Ledesma-García, Janet, Montes Morán, Miguel Ángel, Gurrola, Mayra P, Menéndez Díaz, José Ángel, Arenillas de la Puente, Ana, Arriaga, Luis G |
| المساهمون: | Consejo Mexiquense de Ciencia y Tecnología, Ministerio de Ciencia e Innovación (España), European Commission, Ramírez Montoya, Luis Adrián, Montes Morán, Miguel Ángel, Menéndez Díaz, José Ángel, Arenillas de la Puente, Ana |
| بيانات النشر: | Multidisciplinary Digital Publishing Institute |
| سنة النشر: | 2022 |
| المجموعة: | Digital.CSIC (Consejo Superior de Investigaciones Científicas / Spanish National Research Council) |
| مصطلحات موضوعية: | electro-oxidation, microfluidic fuel cell, microwave heating, unsupported aerogel |
| الوصف: | In this work, unsupported Pd aerogel catalysts were synthesized for the very first time by using microwaves as a heating source followed by a lyophilization drying process and used towards formic acid electro-oxidation in a microfluidic fuel cell. Aerogels were also made by heating in a conventional oven to evaluate the microwave effect during the synthesis process of the unsupported Pd aerogels. The performance of the catalysts obtained by means of microwave heating favored the formic acid electro-oxidation with H2SO4 as the electrolyte. The aerogels' performance as anodic catalysts was carried out in a microfluidic fuel cell, giving power densities of up to 14 mW cm-2 when using mass loads of only 0.1 mg on a 0.019 cm2 electrode surface. The power densities of the aerogels obtained by microwave heating gave a performance superior to the resultant aerogel prepared using conventional heating and even better than a commercial Pd/C catalyst. ; Mexican Council for Science and Technology (CONACYT) through project Ciencia de Frontera Grant no. 845132 and estancia Sabatica Conacyt 2021-2. Grant PID2020-113001RB-I00 funded by MCIN/AEI/ 10.13039/501100011033 and by the European Union NextGenerationEU/PRTR; Grant PCI2020-112039 funded by MCIN/AEI/ 10.13039/501100011033 and by the European Union NextGenerationEU/PRTR. ; Peer reviewed |
| نوع الوثيقة: | article in journal/newspaper |
| اللغة: | English |
| تدمد: | 1996-1944 35207965 |
| العلاقة: | #PLACEHOLDER_PARENT_METADATA_VALUE#; info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-113001RB-I00/ES/DESARROLLO DE NUEVOS MATERIALES DE CARBONO POLIMERICOS PARA EL ALMACENAMIENTO DE ENERGIA EN BATERIAS DE DOBLE ION DE SODIO /; info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PCI2020-112039/ES/MATERIALES NANOESTRUCTURADOS INNOVADORES Y TEJIDOS INTELIGENTES PARA ELECTRODOS DE BATERIAS Y SUPERCONDENSADORES DE NUEVA GENERACION/; Materials (Basel, Switzerland); Publisher's version; Sí; Materials 15(4): 1422 (2022); http://hdl.handle.net/10261/304067Test; http://dx.doi.org/10.13039/501100004837Test; http://dx.doi.org/10.13039/501100000780Test; 2-s2.0-85124897433; https://api.elsevier.com/content/abstract/scopus_id/85124897433Test |
| DOI: | 10.3390/ma15041422 |
| DOI: | 10.13039/501100004837 |
| DOI: | 10.13039/501100000780 |
| الإتاحة: | https://doi.org/10.3390/ma1504142210.13039/50110000483710.13039/501100000780Test http://hdl.handle.net/10261/304067Test https://api.elsevier.com/content/abstract/scopus_id/85124897433Test |
| حقوق: | open |
| رقم الانضمام: | edsbas.12B06B02 |
| قاعدة البيانات: | BASE |
Full Text Finder | تدمد: | 19961944 35207965 |
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| DOI: | 10.3390/ma15041422 |