Enhanced five-photon photoluminescence in subwavelength AlGaAs resonators

التفاصيل البيبلوغرافية
العنوان: Enhanced five-photon photoluminescence in subwavelength AlGaAs resonators
المؤلفون: Zalogina, Anastasiia, Tonkaev, Pavel, Tripathi, Aditya, Lee, Hoo-Cheol, Carletti, Luca, Park, Hong-Gyu, Kruk, Sergey S., Kivshar, Yuri
المصدر: Nano Letters, 2022, 22, 10, 4200-4206
سنة النشر: 2022
المجموعة: Physics (Other)
مصطلحات موضوعية: Physics - Optics
الوصف: Multiphoton processes of absorption photoluminescence have enabled a wide range of applications including three-dimensional microfabrication, data storage, and biological imaging. While the applications of two-photon and three-photon absorption and luminescence have matured considerably, higher-order photoluminescence processes remain more challenging to study due to their lower efficiency, particularly in subwavelength systems. Here we report the observation of it five-photon luminescence from a single subwavelength nanoantenna at room temperature enabled by the Mie resonances. We excite an AlGaAs resonator at around 3.6 um and observe photoluminescence at around 740 nm. We show that the interplay of the Mie multipolar modes at the subwavelength scale can enhance the efficiency of the five-photon luminescence by at least four orders of magnitude, being limited only by sensitivity of our detector. Our work paves the way towards applications of higher-order multiphoton processes at the subwavelength scales enabled by the physics of Mie resonances.
Comment: 18 pages, 5 figures
نوع الوثيقة: Working Paper
DOI: 10.1021/acs.nanolett.2c01122
الوصول الحر: http://arxiv.org/abs/2211.11171Test
رقم الانضمام: edsarx.2211.11171
قاعدة البيانات: arXiv