Cooling Dynamics of a Gold Nanoparticle in a Host Medium Under Ultrafast Laser Pulse Excitation: A Ballistic-Diffusive Approach

التفاصيل البيبلوغرافية
العنوان: Cooling Dynamics of a Gold Nanoparticle in a Host Medium Under Ultrafast Laser Pulse Excitation: A Ballistic-Diffusive Approach
المؤلفون: Rashidi-Huyeh, Majid, Volz, Sebastian, Palpant, Bruno
سنة النشر: 2008
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Materials Science
الوصف: We present a numerical model allowing to determine the electron and lattice temperature dynamics in a gold nanoparticle under subpicosecond pulsed excitation, as well as that of the surrounding medium. For this, we have used the electron-phonon coupling equation in the particle with a source term linked with the laser pulse, and the ballistic-diffusive equations for heat conduction in the host medium. Our results show that the heat transfer rate from the particle to the matrix is significantly smaller than the prediction of Fourier's law. Consequently, the particle temperature rise is much larger and its cooling dynamics is much slower than that obtained using Fourier's law, which is attributed to the nonlocal and nonequilibrium heat conduction in the vicinity of the nanoparticle. These results are expected to be of great importance for interpreting pump-probe experiments performed on single nanoparticles or nanocomposite media.
نوع الوثيقة: Working Paper
الوصول الحر: http://arxiv.org/abs/0806.1613Test
رقم الانضمام: edsarx.0806.1613
قاعدة البيانات: arXiv