دورية أكاديمية
In Situ Growth of PbS/PbI2 Heterojunction and Its Photoelectric Properties
العنوان: | In Situ Growth of PbS/PbI2 Heterojunction and Its Photoelectric Properties |
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المؤلفون: | Shangxun Yang, Jun Han, Jin Zhang, Yingxiu Kong, Huan Liu |
المصدر: | Nanomaterials, Vol 12, Iss 4, p 681 (2022) |
بيانات النشر: | MDPI AG, 2022. |
سنة النشر: | 2022 |
المجموعة: | LCC:Chemistry |
مصطلحات موضوعية: | in situ growth, heterojunction, photoresponse, specific detectivity, wide-spectrum detector, Chemistry, QD1-999 |
الوصف: | In this paper, PbI2 thin films with a uniform surface morphology and compact structure were prepared by adjusting the spin coating process parameters. On such a basis, the PbS/PbI2 heterojunction was fabricated on the PbI2 surface by the method of in situ chemical replacement growth. The results show that the PbS/PbI2 heterojunction grown by this method has a clear interface and is closely combined. The introduction of a PbS layer enables its spectral response range to cover the visible and near-infrared regions. Compared with the PbI2 thin film device, its responsivity is increased by three orders of magnitude, its response time reduced by 42%, and its recovery time decreased by nearly 1/2 under 450 nm illumination. In the case that there is no response for the PbI2 thin film device under 980 nm illumination, the specific detectivity of the PbS/PbI2 heterojunction device still amounts to 1.8 × 108 Jones. This indicates that the in situ chemical replacement is a technique that can construct a high-quality heterojunction in a simple process. PbS/PbI2 heterojunction fabricated by this method has a visible–near-infrared light detection response range, which provides a new idea for creating visible–near-infrared common-path detection systems. |
نوع الوثيقة: | article |
وصف الملف: | electronic resource |
اللغة: | English |
تدمد: | 12040681 2079-4991 |
العلاقة: | https://www.mdpi.com/2079-4991/12/4/681Test; https://doaj.org/toc/2079-4991Test |
DOI: | 10.3390/nano12040681 |
الوصول الحر: | https://doaj.org/article/ce59b3e1709643caa3ec278c85edf6a3Test |
رقم الانضمام: | edsdoj.59b3e1709643caa3ec278c85edf6a3 |
قاعدة البيانات: | Directory of Open Access Journals |
تدمد: | 12040681 20794991 |
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DOI: | 10.3390/nano12040681 |