دورية أكاديمية

Interannual and Seasonal Dynamics of Volatile Organic Compound Fluxes From the Boreal Forest Floor

التفاصيل البيبلوغرافية
العنوان: Interannual and Seasonal Dynamics of Volatile Organic Compound Fluxes From the Boreal Forest Floor
المؤلفون: Mäki, Mari, Aalto, Juho, Hellen, Heidi, Pihlatie, Mari, Bäck, Jaana
المساهمون: Ecosystem processes (INAR Forest Sciences), Department of Forest Sciences, Institute for Atmospheric and Earth System Research (INAR), Department of Physics, Department of Agricultural Sciences, Environmental Soil Science, Methane and nitrous oxide exchange of forests, Viikki Plant Science Centre (ViPS), Forest Ecology and Management
بيانات النشر: Frontiers Media
سنة النشر: 2019
المجموعة: Helsingfors Universitet: HELDA – Helsingin yliopiston digitaalinen arkisto
مصطلحات موضوعية: biogenic volatile organic compound, flux, forest floor, temperature, seasonality, vegetation, decomposition, SCOTS PINE, MONOTERPENE EMISSIONS, ATMOSPHERIC OH, CLIMATE-CHANGE, VOC EMISSIONS, PTR-TOF, SOIL, EXCHANGE, MODEL, METHANOL, 1172 Environmental sciences, 4112 Forestry
الوصف: In the northern hemisphere, boreal forests are a major source of biogenic volatile organic compounds (BVOCs), which drive atmospheric processes and lead to cloud formation and changes in the Earth's radiation budget. Although forest vegetation is known to be a significant source of BVOCs, the role of soil and the forest floor, and especially interannual variations in fluxes, remains largely unknown due to a lack of long-term measurements. Our aim was to determine the interannual, seasonal and diurnal dynamics of boreal forest floor volatile organic compound (VOC) fluxes and to estimate how much they contribute to ecosystem VOC fluxes. We present here an 8-year data set of forest floor VOC fluxes, measured with three automated chambers connected to the quadrupole proton transfer reaction mass spectrometer (quadrupole PTR-MS). The exceptionally long data set shows that forest floor fluxes were dominated by monoterpenes and methanol, with relatively comparable emission rates between the years. Weekly mean monoterpene fluxes from the forest floor were highest in spring and in autumn (maximum 59 and 86 mu g m(-2) h(-1), respectively), whereas the oxygenated VOC fluxes such as methanol had highest weekly mean fluxes in spring and summer (maximum 24 and 79 mu g m(-2) h(-1), respectively). Although the chamber locations differed from each other in emission rates, the inter-annual dynamics were very similar and systematic. Accounting for this chamber location dependent variability, temperature and relative humidity, a mixed effects linear model was able to explain 79-88% of monoterpene, methanol, acetone, and acetaldehyde fluxes from the boreal forest floor. The boreal forest floor was a significant contributor in the forest stand fluxes, but its importance varies between seasons, being most important in autumn. The forest floor emitted 2-93% of monoterpene fluxes in spring and autumn and 1-72% of methanol fluxes in spring and early summer. The forest floor covered only a few percent of the forest stand fluxes in summer. ...
نوع الوثيقة: article in journal/newspaper
وصف الملف: application/pdf
اللغة: English
العلاقة: This research was funded by the Academy of Finland Centre of Excellence Programme (Grant No. 307331), Academy Research Fellow project (Grant No. 2884941), the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme (Grant Agreement No. 757695), and by the Jenny and AnttiWihuri Foundation.; Mäki , M , Aalto , J , Hellen , H , Pihlatie , M & Bäck , J 2019 , ' Interannual and Seasonal Dynamics of Volatile Organic Compound Fluxes From the Boreal Forest Floor ' , Frontiers in plant science , vol. 10 , 191 . https://doi.org/10.3389/fpls.2019.00191Test; ORCID: /0000-0002-6107-667X/work/55059027; ORCID: /0000-0001-6035-3949/work/55062352; ORCID: /0000-0002-9498-2476/work/55063085; 56d87eb8-ff3b-4f4b-80c5-253cb5bea78c; http://hdl.handle.net/10138/299996Test; 000459370000002
الإتاحة: http://hdl.handle.net/10138/299996Test
حقوق: cc_by ; openAccess ; info:eu-repo/semantics/openAccess
رقم الانضمام: edsbas.604804AE
قاعدة البيانات: BASE