يعرض 1 - 5 نتائج من 5 نتيجة بحث عن '"Jiaqi Lin"', وقت الاستعلام: 1.36s تنقيح النتائج
  1. 1
  2. 2

    المصدر: Physical Review Letters. 126

    الوصف: The discovery of superconductivity in a d(9-delta) nickelate has inspired disparate theoretical perspectives regarding the essential physics of this class of materials. A key issue is the magnitude of the magnetic superexchange, which relates to whether cuprate-like high-temperature nickelate superconductivity could be realized. We address this question using Ni L-edge and O K-edge spectroscopy of the reduced d(9-1/3) trilayer nickelates R4Ni3O8 (where R = La, Pr) and associated theoretical modeling. A magnon energy scale of similar to 80 meV resulting from a nearest-neighbor magnetic exchange of J = 69(4) meV is observed, proving that d(9-delta) nickelates can host a large superexchange. This value, along with that of the Ni-O hybridization estimated from our O K-edge data, implies that trilayer nickelates represent an intermediate case between the infinite-layer nickelates and the cuprates. Layered nickelates thus provide a route to testing the relevance of superexchange to nickelate superconductivity.

  3. 3

    المصدر: Physical Review Letters. 124

    الوصف: The discovery of charge-density-wave-related effects in the resonant inelastic x-ray scattering spectra of cuprates holds the tantalizing promise of clarifying the interactions that stabilize the electronic order. Here, we report a comprehensive resonant inelastic x-ray scattering study of La_{2-x}Sr_{x}CuO_{4} finding that charge-density wave effects persist up to a remarkably high doping level of x=0.21 before disappearing at x=0.25. The inelastic excitation spectra remain essentially unchanged with doping despite crossing a topological transition in the Fermi surface. This indicates that the spectra contain little or no direct coupling to electronic excitations near the Fermi surface, rather they are dominated by the resonant cross section for phonons and charge-density-wave-induced phonon softening. We interpret our results in terms of a charge-density wave that is generated by strong correlations and a phonon response that is driven by the charge-density-wave-induced modification of the lattice.

  4. 4

    المصدر: Physical Review Materials. 3

    الوصف: $5d$ iridates have shown vast emergent phenomena due to a strong interplay among their lattice, charge, and spin degrees of freedom, because of which the potential in spintronic application of the thin-film form is highly leveraged. Here we have epitaxially stabilized perovskite $\mathrm{SrI}{\mathrm{r}}_{0.8}\mathrm{S}{\mathrm{n}}_{0.2}{\mathrm{O}}_{3}$ on [001] $\mathrm{SrTi}{\mathrm{O}}_{3}$ substrates through pulsed laser deposition and systematically characterized the structural, electronic, and magnetic properties. Physical property measurements unravel an insulating ground state with a weak ferromagnetism in the compressively strained epitaxial film. The octahedral rotation pattern is identified by synchrotron x-ray diffraction, resolving a mix of ${a}^{+}{b}^{\ensuremath{-}}{c}^{\ensuremath{-}}$ and ${a}^{\ensuremath{-}}{b}^{+}{c}^{\ensuremath{-}}$ domains. X-ray magnetic resonant scattering directly demonstrates a G-type antiferromagnetic structure of the magnetic order and the spin canting nature of the weak ferromagnetism.

  5. 5

    المصدر: Physical Review Letters. 123

    الوصف: While condensed matter systems host both Fermionic and Bosonic quasi-particles, reliably predicting and empirically verifying topological states is only mature for Fermionic electronic structures, leaving topological Bosonic excitations sporadically explored. This is unfortunate, as Bosonic systems such a phonons offer the opportunity to assess spinless band structures where nodal lines can be realized without invoking special additional symetries to protect against spin-orbit coupling. Here we combine first-principles calculations and meV-resolution inelastic x-ray scattering to demonstrate the first realization of parity-time reversal ($\mathcal{PT}$) symmetry protected helical nodal lines in the phonon spectrum of MoB$_{2}$. This structure is unique to phononic systems as the spin-orbit coupling present in electronic systems tends to lift the degeneracy away from high-symmetry locations. Our study establishes a protocol to accurately identify topological Bosonic excitations, opening a new route to explore exotic topological states in crystalline materials.