التفاصيل البيبلوغرافية
| العنوان: |
A cautionary tale: A study of amethane enhancement over the north sea |
| المؤلفون: |
Cain, M, Warwick, NJ, Fisher, RE, Lowry, D, Lanoisellé, M, Nisbet, EG, France, J, Pitt, J, O’Shea, S, Bower, KN, Allen, G, Illingworth, S, Manning, AJ, Bauguitte, S, Pisso, I, Pyle, JA |
| بيانات النشر: |
American Geophysical Union (AGU)
//dx.doi.org/10.1002/2017jd026626
Journal of Geophysical Research |
| سنة النشر: |
2017 |
| المجموعة: |
Apollo - University of Cambridge Repository |
| مصطلحات موضوعية: |
37 Earth Sciences, 3701 Atmospheric Sciences, 3705 Geology, 13 Climate Action |
| الوصف: |
AbstractAirborne measurements of a methane (CH4) plume over the North Sea from August 2013 are analyzed. The plume was only observed downwind of circumnavigated gas fields, and three methods are used to determine its source. First, a mass balance calculation assuming a gas field source gives a CH4 emission rate between 2.5 ± 0.8×104 and 4.6 ± 1.5×104 kg h−1. This would be greater than the industry's reported 0.5% leak rate if it were emitting for more than half the time. Second, annual average UK CH4 emissions are combined with an atmospheric dispersion model to create pseudo‐observations. Clean air from the North Atlantic passed over mainland UK, picking up anthropogenic emissions. To best explain the observed plume using pseudo‐observations, an additional North Sea source from the gas rigs area is added. Third, the δ13C‐CH4 from the plume is shown to be −53‰, which is lighter than fossil gas but heavier than the UK average emission. We conclude that either an additional small‐area mainland source is needed, combined with temporal variability in emission or transport in small‐scale meteorological features. Alternatively, a combination of additional sources that are at least 75% from the mainland (−58‰) and up to 25% from the North Sea gas rigs area (−32‰) would explain the measurements. Had the isotopic analysis not been performed, the likely conclusion would have been of a gas field source of CH4. This demonstrates the limitation of analyzing mole fractions alone, as the simplest explanation is rejected based on analysis of isotopic data. ; The MAMM project was funded by the UK Natural Environment Research Council ... |
| نوع الوثيقة: |
article in journal/newspaper |
| وصف الملف: |
application/pdf |
| اللغة: |
English |
| العلاقة: |
https://www.repository.cam.ac.uk/handle/1810/264998Test |
| DOI: |
10.17863/CAM.10861 |
| الإتاحة: |
https://doi.org/10.17863/CAM.10861Test
https://www.repository.cam.ac.uk/handle/1810/264998Test |
| رقم الانضمام: |
edsbas.C08F00CF |
| قاعدة البيانات: |
BASE |
