دورية
Hetero-Interfaces on Cu Electrode for Enhanced Electrochemical Conversion of CO2to Multi-Carbon Products
| العنوان: | Hetero-Interfaces on Cu Electrode for Enhanced Electrochemical Conversion of CO2to Multi-Carbon Products |
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| المؤلفون: | Li, Xiaotong, Wang, Jianghao, Lv, Xiangzhou, Yang, Yue, Xu, Yifei, Liu, Qian, Wu, Hao Bin |
| المصدر: | Nano-Micro Letters; December 2022, Vol. 14 Issue: 1 |
| مستخلص: | Dual-site electrocatalysts with in situ formed metal-oxide interfaces are proposed and demonstrated to enhance the formation of multi-carbon products from electrochemical CO2reduction.The 0.5-UiO/Cu delivers a high C2+ Faradaic efficiency of over 74% with notably boosted formation rate and durability, surpassing most reported electrocatalysts.A unique mechanism of UiO-66 to induce in situ reconstruction of Cu surface and formation of UiO-66-derived amorphous ZrOx/Cu interface is uncovered, which improves the selectivity and productivity toward C2+ products. |
| قاعدة البيانات: | Supplemental Index |
Full Text Finder | تدمد: | 23116706 21505551 |
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| DOI: | 10.1007/s40820-022-00879-5 |