ACTRIS ACSM intercomparison – Part 1: Reproducibility of concentration and fragment results from 13 individual Quadrupole Aerosol Chemical Speciation Monitors (Q-ACSM) and consistency with co-located instruments
| العنوان: | ACTRIS ACSM intercomparison – Part 1: Reproducibility of concentration and fragment results from 13 individual Quadrupole Aerosol Chemical Speciation Monitors (Q-ACSM) and consistency with co-located instruments |
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| المؤلفون: | Valérie Gros, Laurent Poulain, Stéphanie Verlhac, Nicolas Bonnaire, David C. Green, Philip Croteau, Ari Setyan, Jean-Eudes Petit, M. Bressi, Begoña Artíñano, Andrés Alastuey, Claudio A. Belis, Mikko Äijälä, Jean Sciare, Urs Baltensperger, Fabrizia Cavalli, Francesco Canonaco, Chris Rene Lunder, Roman Fröhlich, Esther Coz, María Cruz Minguillón, Hartmut Herrmann, Liine Heikkinen, John T. Jayne, Anna Ripoll, Véronique Riffault, Manjula R. Canagaratna, André S. H. Prévôt, Olivier Favez, Max Priestman, Alfred Wiedensohler, Michael J. Cubison, Dominique Baisnée, Vincent Crenn, Ettore Petralia, Colin D. O'Dowd, C. Carbone, Wenche Aas, Griša Močnik, Jurgita Ovadnevaite, Jay G. Slowik, Roland Sarda-Esteve, Johanna K. Esser-Gietl |
| المساهمون: | Génie Civil et Environnemental (GCE), École des Mines de Douai (Mines Douai EMD), Institut Mines-Télécom [Paris] (IMT)-Institut Mines-Télécom [Paris] (IMT), Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS), Service de Radiologie [Créteil], CHI Créteil, Norwegian Institute for Air Research (NILU), Institute of Environmental Assessment and Water Research (IDAEA), Consejo Superior de Investigaciones Científicas [Spain] (CSIC), Centro de Investigaciones Energéticas Medioambientales y Tecnológicas [Madrid] (CIEMAT), Paul Scherrer Institute (PSI), JRC Institute for Environment and Sustainability (IES), European Commission - Joint Research Centre [Ispra] (JRC), Angewandte Physik, Universität Paderborn (UPB), National University of Ireland [Galway] (NUI Galway), Laboratoire de Physiologie des Poissons, Institut National de la Recherche Agronomique (INRA), Leibniz Institute for Tropospheric Research (TROPOS), Institut Mines-Télécom [Paris] (IMT), Aerodyne Research Inc., Institut de recherches sur la catalyse et l'environnement de Lyon (IRCELYON), Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS), Department of Physics, Centre for Materials and Processes (CERI MP), Ecole nationale supérieure Mines-Télécom Lille Douai (IMT Lille Douai), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Chimie Atmosphérique Expérimentale (CAE), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Consejo Superior de Investigaciones Científicas [Madrid] (CSIC), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC), Centre for Materials and Processes (CERI MP - IMT Nord Europe), Ecole nationale supérieure Mines-Télécom Lille Douai (IMT Nord Europe), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Université de Lyon-Université de Lyon-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS) |
| المصدر: | Atmospheric Measurement Techniques Atmospheric Measurement Techniques, European Geosciences Union, 2015, 8 (12), pp.5063-5087. ⟨10.5194/amt-8-5063-2015⟩ Crenn, V, Sciare, J, Croteau, P L, Verlhac, S, Fröhlich, R, Belis, C A, Aas, W, Äijälä, M, Alastuey, A, Artiñano, B, Baisnée, D, Bonnaire, N, Bressi, M, Canagaratna, M, Canonaco, F, Carbone, C, Cavalli, F, Coz, E, Cubison, M J, Esser-Gietl, J K, Green, D C, Gros, V, Heikkinen, L, Herrmann, H, Lunder, C, Minguillón, M C, Močnik, G, O'Dowd, C D, Ovadnevaite, J, Petit, J E, Petralia, E, Poulain, L, Priestman, M, Riffault, V, Ripoll, A, Sarda-Estève, R, Slowik, J G, Setyan, A, Wiedensohler, A, Baltensperger, U, Prévôt, A S H, Jayne, J T & Favez, O 2015, ' ACTRIS ACSM intercomparison-Part 1 : Reproducibility of concentration and fragment results from 13 individual Quadrupole Aerosol Chemical Speciation Monitors (Q-ACSM) and consistency with co-located instruments ', Atmospheric Measurement Techniques, vol. 8, no. 12, pp. 5063-5087 . https://doi.org/10.5194/amt-8-5063-2015Test Atmospheric Measurement Techniques, 2015, 8 (12), pp.5063-5087. ⟨10.5194/amt-8-5063-2015⟩ Atmospheric Measurement Techniques, Vol 8, Iss 12, Pp 5063-5087 (2015) ResearcherID Digital.CSIC. Repositorio Institucional del CSIC instname Crenn, V, Sciare, J, Croteau, P L, Verlhac, S, Fröhlich, R, Belis, C A, Aas, W, Äijälä, M, Alastuey, A, Artiñano, B, Baisnée, D, Bonnaire, N, Bressi, M, Canagaratna, M, Canonaco, F, Carbone, C, Cavalli, F, Coz, E, Cubison, M J, Esser-Gietl, J K, Green, D C, Gros, V, Heikkinen, L, Herrmann, H, Lunder, C, Minguillón, M C, Močnik, G, O'Dowd, C D, Ovadnevaite, J, Petit, J E, Petralia, E, Poulain, L, Priestman, M, Riffault, V, Ripoll, A, Sarda-Estève, R, Slowik, J G, Setyan, A, Wiedensohler, A, Baltensperger, U, Prévôt, A S H, Jayne, J T & Favez, O 2015, ' ACTRIS ACSM intercomparison-Part 1 : Reproducibility of concentration and fragment results from 13 individual Quadrupole Aerosol Chemical Speciation Monitors (Q-ACSM) and consistency with co-located instruments ' Atmospheric Measurement Techniques, vol 8, no. 12, pp. 5063-5087 . DOI: 10.5194/amt-8-5063-2015 Crenn, V, Sciare, J, Croteau, P L, Verlhac, S, Froehlich, R, Belis, C A, Aas, W, Äijälä, M, Alastuey, A, Artinano, B, Baisnee, D, Bonnaire, N, Bressi, M, Canagaratna, M, Canonaco, F, Carbone, C, Cavalli, F, Coz, E, Cubison, M J, Esser-Gietl, J K, Green, D C, Gros, V, Heikkinen, L, Herrmann, H, Lunder, C, Minguillon, M C, Mocnik, G, O'Dowd, C D, Ovadnevaite, J, Petit, J-E, Petralia, E, Poulain, L, Priestman, M, Riffault, V, Ripoll, A, Sarda-Esteve, R, Slowik, J G, Setyan, A, Wiedensohler, A, Baltensperger, U, Prevot, A S H, Jayne, J T & Favez, O 2015, ' ACTRIS ACSM intercomparison-Part 1 : Reproducibility of concentration and fragment results from 13 individual Quadrupole Aerosol Chemical Speciation Monitors (Q-ACSM) and consistency with co-located instruments ' Atmospheric Measurement Techniques, vol 8, no. 12, pp. 5063-5087 . DOI: 10.5194/amt-8-5063-2015 NTNU Open Helsingin yliopiston digitaalinen arkisto King's Research Portal NILU Brage Norwegian Open Research Archives DOAJ-Articles |
| بيانات النشر: | Copernicus GmbH, 2015. |
| سنة النشر: | 2015 |
| مصطلحات موضوعية: | Atmospheric Science, SUBMICRON AEROSOLS, Analytical chemistry, Environmental engineering, 114 Physical sciences, Chloride, chemistry.chemical_compound, Earthwork. Foundations, Nitrate, PARTICULATE MATTER, Calibration, medicine, Organic matter, lcsh:TA170-171, Sulfate, [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces, environment, ORGANIC AEROSOL, 1172 Environmental sciences, [SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, chemistry.chemical_classification, Reproducibility, SIZE DISTRIBUTIONS, lcsh:TA715-787, TA715-787, lcsh:Earthwork. Foundations, METROPOLITAN-AREA, TA170-171, Particulates, MULTIWAVELENGTH AETHALOMETER, lcsh:Environmental engineering, Aerosol, DOWNTOWN ATLANTA, SOURCE APPORTIONMENT, chemistry, MASS-SPECTROMETER DATA, HIGH-RESOLUTION, medicine.drug |
| الوصف: | As part of the European ACTRIS project, the first large Quadrupole Aerosol Chemical Speciation Monitor (Q-ACSM) intercomparison study was conducted in the region of Paris for 3 weeks during the late-fall - early-winter period (November-December 2013). The first week was dedicated to the tuning and calibration of each instrument, whereas the second and third were dedicated to side-by-side comparison in ambient conditions with co-located instruments providing independent information on submicron aerosol optical, physical, and chemical properties. Near real-time measurements of the major chemical species (organic matter, sulfate, nitrate, ammonium, and chloride) in the non-refractory submicron aerosols (NR-PM1) were obtained here from 13 Q-ACSM. The results show that these instruments can produce highly comparable and robust measurements of the NR-PM1 total mass and its major components. Taking the median of the 13 Q-ACSM as a reference for this study, strong correlations (r2 > 0.9) were observed systematically for each individual Q-ACSM across all chemical families except for chloride for which three Q-ACSMs showing weak correlations partly due to the very low concentrations during the study. Reproducibility expanded uncertainties of Q-ACSM concentration measurements were determined using appropriate methodologies defined by the International Standard Organization (ISO 17025, 1999) and were found to be 9, 15, 19, 28, and 36 % for NR-PM1, nitrate, organic matter, sulfate, and ammonium, respectively. However, discrepancies were observed in the relative concentrations of the constituent mass fragments for each chemical component. In particular, significant differences were observed for the organic fragment at mass-to-charge ratio 44, which is a key parameter describing the oxidation state of organic aerosol. Following this first major intercomparison exercise of a large number of Q-ACSMs, detailed intercomparison results are presented, along with a discussion of some recommendations about best calibration practices, standardized data processing, and data treatment. |
| وصف الملف: | application/pdf |
| تدمد: | 1867-8548 1867-1381 |
| الوصول الحر: | https://explore.openaire.eu/search/publication?articleId=doi_dedup___::8735b269c2bdc70e202e40d436bb2a69Test https://doi.org/10.5194/amt-8-5063-2015Test |
| حقوق: | OPEN |
| رقم الانضمام: | edsair.doi.dedup.....8735b269c2bdc70e202e40d436bb2a69 |
| قاعدة البيانات: | OpenAIRE |
| تدمد: | 18678548 18671381 |
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