دورية أكاديمية

Computer simulation of thermal processes involving Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere

التفاصيل البيبلوغرافية
العنوان: Computer simulation of thermal processes involving Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere
المؤلفون: Barbin,Nikolay, Titov,Stanislav, Terentiev,Dmitry, Kobelev,Anton
المصدر: Nuclear Energy and Technology 9(4): 273-279
بيانات النشر: National Research Nuclear University MEPhI (Moscow Engineering Physics Institute)
سنة النشر: 2023
المجموعة: Pensoft Publishers
مصطلحات موضوعية: thermodynamic simulation, thermal processes, equilibrium constant, radionuclides, radioactive graphite, heating, air atmosphere
الوصف: The paper presents the results from a thermodynamic analysis of the behavior of Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere. The TERRA software package was used for the thermodynamic analysis in a temperature range of 300 to 3600 K to determine the possible composition of the ionized, gaseous and condensed phases. It has been found that strontium is in the form of condensed SrCl2(c) and gaseous SrCl2 in a temperature range of 300 to 1600 K, and in the form of gaseous SrCl2, SrO, SrCl and Sr and ionized SrCl+, Sr+ and SrO+ when the temperature is increased from 1600 to 3600 K. Calcium is in the form of condensed CaCl2(c), CaUO4(c), CaO(c) and gaseous CaCl2 in the temperature interval between 300 and 2100 K, and in the form of gaseous Ca, CaCl and CaO and ionized Ca+, CaO+ and CaCl+ when the temperature is increased from 2100 to 3600 K. The paper determines the key reactions within individual phases and among condensed, gaseous and ionized phases. The equilibrium constants of their reactions have been calculated. Based on the results obtained, dependence plots are presented for the Sr and Ca radionuclide distribution by phases.
نوع الوثيقة: article in journal/newspaper
وصف الملف: text/html
اللغة: English
العلاقة: info:eu-repo/semantics/altIdentifier/eissn/2452-3038
DOI: 10.3897/nucet.9.116661
الإتاحة: https://doi.org/10.3897/nucet.9.116661Test
https://nucet.pensoft.net/article/116661Test/
حقوق: info:eu-repo/semantics/openAccess ; CC BY 4.0
رقم الانضمام: edsbas.3A55C8F7
قاعدة البيانات: BASE