دورية أكاديمية

Transition from a uni- to a bimodal interfacial charge distribution in LaAlO3/SrTiO3 upon cooling.

التفاصيل البيبلوغرافية
العنوان: Transition from a uni- to a bimodal interfacial charge distribution in LaAlO3/SrTiO3 upon cooling.
المؤلفون: Zwiebler, M., Di Gennaro, E., Hamann-Borrero, J. E., Ritschel, T., Green, R. J., Sawatzky, G. A., Schierle, E., Weschke, E., Leo, A., Granozio, F. Miletto, Geck, J.
المصدر: Scientific Reports; 10/27/2020, Vol. 10 Issue 1, pN.PAG-N.PAG, 1p
مصطلحات موضوعية: X-rays, ATOMIC layer deposition, COOLING, TITANIUM oxides, ELECTRONS
مستخلص: We present a combined resonant soft X-ray reflectivity and electric transport study of LaAlO 3 / SrTiO 3 field effect devices. The depth profiles with atomic layer resolution that are obtained from the resonant reflectivity reveal a pronounced temperature dependence of the two-dimensional electron liquid at the LaAlO 3 / SrTiO 3 interface. At room temperature the corresponding electrons are located close to the interface, extending down to 4 unit cells into the SrTiO 3 substrate. Upon cooling, however, these interface electrons assume a bimodal depth distribution: They spread out deeper into the SrTiO 3 and split into two distinct parts, namely one close to the interface with a thickness of about 4 unit cells and another centered around 9 unit cells from the interface. The results are consistent with theoretical predictions based on oxygen vacancies at the surface of the LaAlO 3 film and support the notion of a complex interplay between structural and electronic degrees of freedom. [ABSTRACT FROM AUTHOR]
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قاعدة البيانات: Complementary Index
الوصف
تدمد:20452322
DOI:10.1038/s41598-020-74364-7